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The paper describes the quantized Hamilton dynamics (QHD) approach that extends classical Hamiltonian dynamics and captures quantum effects, such as zero point energy, tunneling, decoherence, branching, and statespecific dynamics. The approximations are made by closures of the hierarchy of Heisenberg equations for quantum observables with the higher order observables decomposed into products of...
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ژورنال
عنوان ژورنال: Structural Chemistry
سال: 2016
ISSN: 1040-0400,1572-9001
DOI: 10.1007/s11224-015-0738-x